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ORNL-4528.txt
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Dw - /50 |
. -UC-80 — Reactor Technology
E '_: ', ‘_ TWO-FLUID MOLTEN-SALT BREEDER REACTOR
' DESIGN STUDY (STATUS AS 0|= JANUARY 1, 1958)"]‘ _‘
_-R Robertson 0 L Smith e
- .R.B Brlggs ~E s Bettis SRR
AL T e o
.'.'?,‘.-:_EOAK RIDGE NA'I'IONAI. LABORA'I'ORY
: operaled by
umou CARB!DE CORPORATION
L for the o ST
u s A'I'OMlC ENERGY commss:on -
. DISTRIBUTION OF THIS DOCUMENT IS UNLIMITED
&
Prlnted in the Umfed Sfu!es of Amerlca. Avalluble from Clearmghouse for Federol
Scientific and Techmcol lnformahon National Bureau of Stcndards, R
7 U s. Depurfment of Commerce, Sprlngfneid Virginia 22151 - s
Prlce° Prmted Copy $3 00; Mrcrof‘che $O 65 L S
- Thus report was prepared as on account of Government sponsored work. Neithe;‘ th'e_ Un'ifedVStefr:esr,_;
“mor. the Comm:sslon, nor-any person acting on behalf of the Commissuon." .
" As. used in the above, * ‘person acting on behalf of the Commission®’ andudes any employee oF .~
: contrucfor of the Commission, or empioyee ‘of such confructor, to the- extent fhof such. employee 1
or . conlracfor of the Commnss:on, or_employee of such confructor prepares, dlssemma?es, or>
: provvdes access to, any mformuhon pursucmf to hns employmenf or comruc! wnh Ihe Commussnon,
'_. LEGAL: NOTICE -
<AL Mukes ony wurrnnty or represenfuhon, expressed or lrnphod with respect to the uccurocy, ey
complefeness, of usefulness of the mformuhon contained in this report, or lhot the ‘use of
ony mformahon, uppamfus, meihod or process dlsclosed in thls reporf rnuy not mfnnge
pnvately owned rights; or ~ . s :
'B Assumes any habuhhes with respect to fhe use of, or for damuges resulhng from fhe use of-'—_' o
cny mformahon, apparatus, mefl\od or process disclosed in this report, .
or his emp!oyment wnth such contruc#or.
g ' ORNL-4528
' UC-80 — Reactor Technology
»
"
Contract No, W-7405-eng-26
|
REACTOR DIVISION
TWO-FLUID MOLTEN-SALT BREEDER REACTOR DESIGN STUDY (STATUS AS OF JANUARY 1, 1968}
R. C. Robertson 0. L. Smith
R. B. Briggs E. S. Bettis
A
-
v LEGAL NOTICE
This report was prepared as an account of work
sponsored by the United States Government. Neither
the United States nor the United States Atomic Energy
Commission, nor any of their employees, nor any of
their contractors, subcontractors, or their employees,
makes any warranty, express or implied, or assumes any
legal Hlability or responsibility for the accuracy, com-
pleteness or usefulness of any information, apparatus,
product or process disclosed, or represents that its use
would not infringe privately owned rights. :
AUGUST 1970 -
OAK RIDGE NATIONAL LABORATORY
QOak Ridge, Tennessee
operated by
UNION CARBIDE CORPORATION
~ for the
fi\ U.S. ATOMIC ENERGY COMMISSION
o
b=
w
DISTRIBUTION OF THIS DOCUMENT IS UNLIMITED
(A
»
o
a4/
CONTENTS
N 3T T U 1
1. Introduction ISR 2
2. Résume of Design Considerations . .........ueeuneeenrnneeeeernnreeeoennaresnnnnecesennenns 2
3, Materials ... i i e i e e et ettt et i 6
30 Gemeral ... s 6
B2 1 S 7
K 0 T 5 P13 - | ()20 . 11
34 Graphite ............oiiiiiiiiiia, e 12
3.5 Graphite-to-Metal Joints .. ... ...ttt ittt i i i it e 14
4. General Plant Description and FLOWSHEELS - -+« v e v eee e e e e e e e e e e e e e e e e et e et 16
0 T € 1T Y PP 16
B SIE ittt it i e e ettt i it e 16
43 Reactor Plant . ... ... i i i i it i it i i it e i et 18
44 TurbinePlant ................... e ettt etee e te et a et e e 26
4.5 Salt ProcessingPlant..................... e P 29
5. Major COmPOnents . ...........uinutiint it e 32
5.1 Reactor ....c.onininii 32
5.2 Fuel Salt Primary Heat Exchanger ............ e, S s 40
5.3 Blanket Salt Primary Heat Exchanger ................... T 42
54 SaltCirculatingPumps ...........c.ciieiennnnnan.. fereererenese e e eireeeaaaa. 44
55 OffGasSystem ................c.o.... Ceneeae . 48
56 DrainTanks ..........ccoiiiiiiinnnnnnn. feevsene e et aaeead e esaneaas 49
ST SHEAM GEMETALONS - . . e« v e s e ve e seene e ee e eaa e e e e e e e e e e e e e e e et e e e e 53
58 SteamReheaters....................... e e e hireaeas e et 53
- 59 Reheat Steam Preheaters S e et eeaenas 57
5.10 Maintenance . .......... ettt eeeenans e S s T 57
6. Reactor Physics and Fuel Cycle Analysis . ... eeenaen .............. 60
6.1 Optimization of Reactor Parameters .............. e 60
6.2 Useful Life of Moderator Graphite . . e e e et tiess et aaeaenaas 63
63 Flux Flattening ................. e, T 66
64 Fuel Cell Calculations . .. . .. ... e, SR e 67
6.5 Temperature Coefficients of Reactivity .......... ..., e 68
- 6.6 Dynamics Analysis 70
111
iv
7. Cost Estimates .. ............ £ttt eesenneanas et eieeetisnesenaneassnesannaseenaneaannaae 71
T GNEIAl « v v v e e e e, . 71
7.2 Construction Costs ...... v eeesatecensneea e et 71
7.3 Power Production Costs ........................ e it eeseseseseaenaes 73
Appendix.A': Cost Estimates ............. e beateacearaaeecaaceatarenetenonrrasenaan e ... 5
"
€A -
"
¥)
&/ »
TWO-FLUID MOLTEN-SALT BREEDER REACTOR DESIGN STUDY
(STATUS AS OF JANUARY 1, 1968) '
R. C. Roberts‘on . 0 L. Smith
'R. B. Briggs E. S. Bettis
ABSTRACT
A conceptual design study of e 1000-Mw(e) thermal breeder power station based on a two-fluid -
MSBR was commenced in 1966 as part of a program to determine whether a molten-salt reactor using
the thonum— U fuel cycle could produce electric power at sufficiently low cost to be of interest and
at the same time show good utilization of U.S. nuclear fuel resources. This report covers the progress
- made in the study up to August 1967, at which time the two-fluid MSBR work was set aside in order
to study a single-fluid MSBR concept. The latter became of interest at that time due to the discovery
that protactinium and other fission products could be separated from a uxanmm-and-thonum-bearing
_ fuel salt by reductive extraction into liquid bismuth.
The two-fluid MSBR is graphrte-moderated and: -reflected, with a 7L1F-BeF2-UF4 fuel salt
~ circulated through the core and a LiF—ThF4-BeF2 blanket salt circulated through separate flow
channels distributed throughout the core, as well as in a surroundmg undermoderated region. The
fissrons raise the temperature of the fuel salt to about 1300 °F and that of the blanket salt to about -
1250°F. Heat is removed from the salts in shell—and-tube heat exchangers to raise the temperature of a
circulating NaBF4-NaF coolant salt to about 1150 F The coolant salt transports the heat to steam
generators and ‘reheaters to prov:de 3500-psia 1000 FllOOO F steam for a conventronal turbine-
generator.
The conceptual desxgn was based on use of four reactors and the associated heat transfer systems
in a so-called modular arrangement to supply steam to a single turbine-generator, This made it
- practical to consider replaeement of an entire reactor vessel assembly after the core graphite received
its allowable exposure to neutrons, The total fluence at which it Was thought that addmonal graphite
- dimensional changes would become excessive was taken as 3 X 10% neutrons/cm (E > 50 kev), or -
about eight years of full-power operation, _
All portions of the systems in contact with the fluoride or fluoroborate salts would be fabnmted
" of Hastelloy N that has a small amount of titanium added to improve the resistance to radiation
damage. The graphite would be a specially coated grade having low gas permeability to xenon and
better resistance to radiation damage than conventional material. The two-fluid concept involves
' _ joining graphite core elements to Haételloy N tubing using a brazing process developed at ORNL.
The reactors and associated systems would be housed in concrete cells to provrde biological
~ shielding and double containment of all radxoact:ve materials.
Plant flowsheets and layouts were developed sufficiently during the study to give an indication of
- feasibility and to give a basis for cost estimates, but no optimization studies were made. Safety aspects
were considered throughout the design effort, but no formal safety analysis was completed. .
. Fuel and blanket salts would be continuously processed in a nearby cell to remove fission products
and to recover the bred product. The processing rate would correspond to removal of uranium and
~ protactinium from the blanket on a 3-day cycle and rare-earth fission products from the core on a
60-day cycle. Since no conceptual designs for the chemical plant were completed, cost estimates could
-not be on a definitive basis. The tentatively estimated fuel-cycle cost is about 0.5 mill/kwhr, which
includes the fixed charges and operating costs for the processing equipment, the fuel inventory charge,
- -and the credit for bred fuel Graphxte replacement costs, which are not included, would add about 0.2
) rmrlllkwhr
The tentatively estimated total construction cost of a lOOO—Mw(e) MSBR stat:on ‘based on the
- early 1968 value of the dollar, is about $141 per kilowatt. The power production cost for a privately
owned station, based on fixed charges of 13,7% and 80% plant factor, is about 4 mills/kwhr, The net
- thermal efficiency of the plant would be about 44 9%. ,
~ The off-gas, fuel processing, afterheat removal, “and mamtcnance systems needed further
investigation at the time the study was suspended, and the limited performance of the graphite
- undoubtedly restricts the design and imposes a maintenance penalty, but the study did not disclose
any aspects which indicated that major technological discoveries would be required to design a two-
¢ fluid molten-salt reactor power station. The major concern was whether mechanical failure of graphite
- tubes in the reactor core would cause the effective lifetime of the core to be slgmficantly less than the
eight years m\posed by the effects of irradiation on the graphite.
1. INTRODUCTION
The basic objective of the Molten-Salt Reactor Pro-
gram is to develop the technology for economical
nuclear power reactors that make use of fluid fuels
which are solutions of fissile and fertile materials in
suitable carrier salts. A major goal is to achieve a
thermal breeder reactor based on the thorium-223U
fuel cycle that will produce power at low cost while
conserving and extending the nation’s fuel resources.
Conceptual design studies of a variety of molten-salt
breeder reactors for large plants are an important part
of this program. In August 1966 we published a survey
report, ORNL-3996,! in which we described briefly the
status of molten-salt reactor technology and the designs
of reactors and fuel processing facilities for 1000-Mw(e)
- power stations. This survey led us to conclude that the
- two-fluid reactor which separates the fuel and blanket
salts held the most promise for development as a -
breeder reactor. The modular version, consisting of four
reactor modules and associated intermediate systems -
supplying steam to one turbme-generator, was selected
for more detailed analysis.
The study of the modular design of a 1000-Mw(e)
plant was begun in the fall of 1966, and some of the
results were published in the MSRP progress reports,
' ORNL-4037,> ORNL4119,2 and ORNL4191.* Much
of the effort was spent on designs for the core and in
exploring the effects of radiation-induced damage to
graphite on the core designs. The plant layout, the cell.
designs, the drain tank systems, the nuclear character-
istics, the maintenance, and the cost estimates were also
examined in more detail than had been possible in the
earlier survey.
Considerable progress had been made in these studxes
when, in August 1967, encouraging information ob-
tained from research on the processing of moltensalt.
fuels indicated that protactinium and some fission
products could be separated from the uranium-and-
thorium-containing fuel salt of a one-fluid reactor by
reductive extraction into liquid bismuth. At about this
same time, nucleéar calculations indicated that a conver-
sion ratio greater than 1 could be achieved in a
1Paul R. Kasten, E, S, Bettis, and Roy C. Robertson, Design
Studies of 1000-Mw{e} Molten-SaIt Breeder Reactors, ORNL-
3996 (August 1966). _
2MSR Program Semiann,” Progr Rept. Aug 31, 1 966
ORNL-4037.
SMSR Program Semiann, Progr Rept. Feb, 28, 1967, ORNL-
4119,
*MSR Program Semiann. Progr. Rept. Aug 31 1967,
ORNL-4191,
one-fluid reactor of acceptable dimensions by increasing
the fuel-salt-to-graphite ratio in the outer regions of the
core. The one-fluid breeder is mechanically simpler than
the two-fluid breeder because it involves only one salt
stream, which contains both the fissile (*?3U) and the
fertile (thorium) constituents. Also, the one-fluid
breeder is a direct descendant of the one-fluid Molten-
_ Salt Reactor Experiment, which has operated well at
Oak Ridge National Laboratory. The attractive pos-
sibility of being able to progress in a direct path from
the MSRE to large thermal breeder reactors of similar
design led us to set aside the studies of two-fluid -
‘breeders to examine one-fluid breeder reactors in equal
detail. The studies of the one-fluid breeders were begun
in September 1967 and are continuing.
Although the one-fluid breeder has the desirable
features mentioned above, the fact remains that the
two-fluid MSBR is inherently capable of achieving a
significantly higher breeding performance. This feature
alone will sustain interest in the two-fluid system. It is
thus important to document the progress made in the
two-fluid breeder study before it was set aside. Present-
ing this information adequately is difficult, because
several months of studies of the one-fluid reactor have
changed some of our ideas about MSBR design, and
new data relevant to the two-fluid reactor have con-
~ tinued to come from the research and development
program. For example, the physical properties of the
salts have a profound influence on the design, yet many
of these properties are under continuous study and
adjustment. Some of the new information will be
mentioned briefly, but the reader should understand
that this report does not fully represent current ideas
‘and that some designs and conceptual drawings pre-
sented here would be considerably altered if they were
to be reexamined on the basis of today’s knowledge.
The studies upon which this report is based involved
personnel from almost all the divisions of ORNL, but
~ particularly those from the Reactor Division, Reactor
Chemistry Division, Chemical Technology Division, the
Metals and Ceramics Division, and the General Engi-
neering Division. A group composed of members of
these divisions, under the leadership of E. S. Bettis,
provided the conceptual designs and data which are
basic to the report.
2. RESUME OF DESIGN CONSIDERATIONS
Several basic considerations influenced our choice of
a two-fluid MSBR concept and many of the details of
the plant design. They are reviewed here to provide the
<
"
A\
reader with a better understanding of the de31gn that
evolved.
A simplified diagram of a two-fluid breeder reactor is
shown in Fig. 2.1. The core of the reactor consists of an
array of tubular graphite elements in the center of the
reactor vessel. A molten fuel salt is recirculated through
the graphite elements and through a shell-and-tube heat
exchanger by means of a centrifugal pump. A molten
blanket salt is similarly recirculated through the space
around and between the graphite pieces in the reactor
vessel and through an external heat transport circuit.
Heat generated in the reactor is transferred from the
fuel and blanket salts to a coolant salt in the heat
exchangers. The coolant -salt is recirculated through
steam generators where the energy is used to convert
the feedwater into superheated steam that drives a
conventional turbinegenerator to produce electricity.
The MSBR is a thermal breeder reactor that is
intended to attain the highest breeding performance
consistent with producing power at low cost. Our past
studies have indicated that a good measure of the
BLANKET-SALT FROM
PROCESSING PLANT . P
BLANKET-SALT l
ll . CRCULATION - . . _
BLANKET-SACT ; ¥ I .
TO PROCESS- = TUBES
ING PLANT
1125°F
COOLANT-SALT TO
STEAM GENERA-~
- REACTOR
TORS i
BLANKET-SALT
HEAT EXCHANGER
1eF N
/ N
COOLANT-SALT FROM MEO°F :
FUEL-SALT HEAT o t
EXCHANGER
performance of a breeder system is the total quantity of
fissionable material that must be mined in order to
provide the fissile inventory for a large nuclear power
system. This total ore requirement should be low. The
terms that describe the performance vary with the
~assumed growth rate of the nuclear electrical industry
and the types of reactors that precede and accompany
the breeders, but in the range of interest the per-
formance of a breeder is approximately proportional to
the product of the breeding gain G and the reciprocal
of the square of the specific inventory, 1/S?. The
“conservation coefficient” G/S? for MSBR’s can be
expected to be in the range of 0.02 to 0.10, where the
specific inventory has units of kilograms of fissionable
‘material per megawatt of electnclty and the breeding
gain is dimensionless.
A practical thermal breeder reactor can only be
fueled on the thorium-232U cycle, and it has a small
potential breeding gain. Typically, n for an MSBR is
'2.22 neutrons produced per neutron absorbed in fissile
material that is an equilibrium mixture of ??>*U and
ORNL-DWG 69-6868
g
2
8
8
GRAPHITE
= | _~~ HELIUM FROM
A
H~ OFF-GAS SYSTEM
FUEL~SALT CIRCULATION PUMP
FUEL-SALT FROM
-a— PROCESSING PLANT |
—= FUEL-SALT TO
PROCESSING
- PLANT
/
f
I E
— i
=
o J
1M1°F
AR
- %’*\W 'OOO‘,FJ | EOARKET- SS‘?QIE T
DRAIN LINE TO BLANKET- -— -
" SALT DRAIN TANKS HE}-_'%XSTO { HEAT EXCHANGER
' SYSTEM GAs SEPARATOR
© FUEL-SALT
HEAT EXCHANGER
- ' COOLANT-SALT FROM
DRAIN LINE 10 - STEAM GENERATORS.
- DRAIN TANKS * 850°%F - -
‘Fig. 2.1. Simplified Flow Diagram of Two-Fluid MSBR,
235, Absorptlon of one neutron in fissile material
and one in fertile material leaves 0.22 of a neutron for
losses to _moderator, carrier salt, leakage, Iughgr iso-
topes, protactinium, fission products, and structural ma-
terials and for absorption in thorium to produce the
gain in 233U,
Achieving high performance in a breeder depends on
keeping the parasitic absorption of neutrons and the
spec1fic inventory of fissile material low. Losses to
carrier salt, moderator, and structural materials and the
rate and cost of processing to keep the fission product
losses low all décrease with increasing concentration of
'uranium in the fuel salt and increasing inventory in the
reactor core. The specific inventory, however, includes
the iventory in the heat transfer equipment external to
the reactor vessel, in storage, and in the fuel processing
plants, so that the specific inventory and the total
inventory cost increase rapidly with increasing concen-
tration of uranium in the fuel salt. The breedmg gain
~and specific inventory must be balanced to obtain the
highest breeding performance (large G/S?) that is
consistent with producing power at low cost.
- The favored fuel salt contains about 0.2 mole % UF,,
of which about 70% is 223U and 35U, 23% is 234U,
and 7% is 236U. The uranium fluoride is dissolved in a
"LiF-BeF, (67-33 mole %) carrier salt. As shown in
Table 3.1, this salt has a liquidus temperature of about
840°F and good flow and heat transfer properties at the
working temperatures. It also has excellent thermal and
radiation stability and, with the use of ?Li, a low cross
section for the parasitic absorption of neutrons. A
ThF,-? LiF-BeF, salt (27-71-2 mole %), which melts at
about 1040°F, is a good choice for the blanket salt. The
physical properties of this salt are also shown in Table
3.1.
Although lithium and beryllium nuclei are good
moderators for neutrons, the moderating properties of
- the fluoride salts are not sufficiently good, when
compared with their neutron absorbing properties, to
build a thermal breeder without the use of other
moderator. Graphite is the best ‘material for this
purpose, because it has good moderation properties, a
low neutron absorption cross section, and good struc-
tral properties at high temperature and can be used in
direct contact with molten fluoride salts.
The design and performance of the reactor depend
considerably on the effects of fast neutrons on the
graphite. Neutron irradiation causes graphite to change
dimensions and its physical properties to deteriorate.
The life of the graphite is expected to be limited to
some total exposure to fast neutrons and therefore to
vary inversely with the maximum power density in the
core. Selection of a design power density for the core
must be based on a balance between the costs of fuel -
inventory, periodic replacement of the graphite, and
other factors that reflect on the net cost of the
electricity produced.
In order for the graphite to have an acceptable
radiation hfe we estimate that the maximum power
density should not exceed about 100 kw per liter of
core volume, With this limit on power density, the core
of a centralstation power reactor would have a volume
of several hundred cubic feet. This size is too large for
- the core to consist of graphite bars and highly enriched
fuel salt contained in a thin metal shell and surrounded
by a region of blanket salt. The critical concentration of
?23U in the fuel salt would be so low that the
absorptions in the carrier salt and the graphite would be
_excessive. Absorption of neutrons by the shell would
- further degrade the performance. '
The concentration of 233U in the fuel salt can be
naised to the desired level by dispersing blanket salt
throughout the core. This is accomplished by making
the graphite moderator in the form of tubular elements
and flowing the fuel salt through the elements and the
blanket salt around the elements. The core composition
is obtained by optimizing the relative volumes of fuel
salt, blanket salt, and graphite within bounds imposed
by limits on the concentration of thorium in the
blanket salt and by the engineering of the core.
" Results of many calculations have shown that the
combined neutron losses to fuel and blanket carrier
salts, the graphite moderator, and higher isotopes will
be near 0.11 in an optimized reactor, leaving 0.11 for
other losses and the breeding gain. Leakage losses are
reduced to a small amount by a thorium blanket of
reasonable thickness around the core. The losses due to
protactinium are kept small by keeping its concen-
tration in the blanket salt low. This is accomplished by
having a blanket of large volume at low neutron flux or
by removing the protactinium from the blanket salt on
a few-day cycle and allowing it to decay in the
processing plant. Xenon-135 must be removed from the
fuel salt on a few-second cycle, or the surfaces of the
graphite elements must be sealed to greatly reduce the
rate of diffusion of xenon into the pores. Most of the -
other fission products must be removed by processing
the fuel salt on a 30-to 50-day cyde. Limiting the total
of the above losses to 0.03 ‘to 0.07 appears to be
reasonable; this leaves a potential breeding gain of 0.04
to 0.08. |
A reactor with a breeding gain in this range and a
specific inventory of 1.5 kg/Mw(e) or less will have
good breeding performance. In order to have this low a
a)
”
r
specific inventory, the amount of 233U external to the
reactor core must be kept to a minimum. The heat
transfer circuit of the reactor must be closely coupled
‘to the reactor vessel, and it must have high perform-
ance. The fissile inventory in the blanket systems must
be kept small by extracting the bred 223U from the
blanket salt on a few-day cycle and making it available
for adding to the fuel salt to compensate for burnup.
Processing the fuel and blanket salts at the reactor site
_is necessary to avoid inventory in transport and storage,
and short cooling- time is important in reducing the
inventory in processing. The processes must be simple
and involve few changes in the physical or chemical
nature of the salts if they are to be carried out rapidly
and inexpensively. Fluorination to remove the uranium
as the volatile UF¢ followed by vacuum distillation to
separate the carrier salt from the rare-earth fission
products satisfies these requirements for processing the
fuel salt. Fluorination to remove the uranium or
extraction of protactinium and uranium into molten
bismuth can satisfy the requirements for the blanket.
With thorium blanket salt dispersed throughout the
core, the breeding gain is largely independent of the size
of the core, but this arrangement imposes several
conditions on the design. The first of these is that
graphite elements must be joined to metal-piping in the
reactor vessel. A perfect separation between the fuel
and blanket salts is not essential to the safety of the
operation, but the leakage must not be so great as to
~ put an excessive burden on the processing facilities.
Processing considerations lead to a preference for any
leakage to be blanket salt into fuel salt, and the leakage
must be kept below about 1 ft*/day in a 1000-Mw(e)
plant. Such a plant would have several hundred graph-
ite-to-metal joints. Our experience led us to choose
graphite-to-metal brazing as the method for obtaim‘ng
adequate leak-tightness.
The graphite elements for the core must be of a size
and shape that are within the capability of manufac-
turers to make and inspect for reasonable cost and with
good quality control. Isotropic material appears de-
sirable and may be essential from the standpoint of
irradiation effects. Thicknesses of sections must be
limited so that the temperature rise due to heating in
the graphite is not large. Effects of irradiation increase
with temperature, and stresses increase with tempera-
ture difference, so a large rise in internal temperature
could result in a large decrease in service life of the core
elements. Graphite tubés 6 in. or less in diameter and
~with a wall % in. or less in thickness appear to fulfill all -
these requirements.
Neutron irradiation produces substantial changes in
length of the graphite elements, and the difference in
expansion of the graphite and the metal parts of the
reactor vessel with temperature changes can also be
~ large. These effects must be accommodated without
overstressing the graphite. We propose to accomplish
this by making the graphite elements in the form of
concentric tubes connected to the reactor vessel at only
one end in order to provide freedom for axial expansion
and contraction. The fuel salt would flow in and out at
the same end of the elements, and the connections
would be to tube sheets at the bottom of the reactor
vessel to allow the salt to drain completely.
Because of the irradiation effects, the graphite tubes
will have to be replaced periodically. Also, one could
expect an occasional failure of a graphite element or a
graphite-to-metal joint from other causes. The reactor
vessel and internals will be highly radioactive after a
short time at high power, and with the graphite
elements brazed to a tube sheet in the bottom of the
reactor vessel, individual tubes could not be readily
- inspected or replaced. We concluded that the most
practical way to renew the graphite in the core would
be to replace the entire reactor vessel and its contents,
Suitable provisions would be required for remotely
operated tools and viewing equipment to cut, weld, and
inspect joints in the piping system. Provisions for
handling and disposing of spent reactor vessels would
have to be included in the plant.
The high melting temperatures of the salts make it .
necessary to preheat the reactor equipment to high
temperature before introducing the salts and to main-
tain the temperature when they are present. The special
problems of maintenance and inspection of the reactor
equipment after it has become radioactive led to our
proposals to install the reactor systems in heated cells,
which are comparable to large furnaces, rather than to
apply heaters and insulation to the vessels and piping.
In our studies of designs for molten-salt breeder
reactors, we are concerned primarily with power sta-
~ tions having outputs of 1000 Mw(e) or more. The
capacities of salt circulation pumps, heat exchangers,
steam generators, etc., needed for such plants are
greater than could reasonably be designed into single
units. In the 1000-Mw(e) MSBR design described in
ORNL-3996,! ‘we chose to connect four primary heat
removal circuits to one reactor vessel, to provide one
coolant and steam generator circuit for each primary
heat removal circuit, and to send the steam from all the
steam generators in the plant to one turbine.
Since the two-fluid breeder has a blanket of low 233U
and high thorium content around the core to capture
the leakage neutrons, reactors of this type can have
about the same breeding performance over a wide range
of size if the maximum power density in the core is
held constant. These facts, together with the special
problems and time required to replace a reactor vessel,
led us to consider a modular design for the two-fluid
MSBR in which. separate, but smaller, reactor vessels
would be coupled to primary heat removal circuits to
provide four autonomous reactor systems delivering
steam to -one -turbine-generator. This modular plant
would be slightly larger than the integral plant, since
four small reactor vessels with associated control sys-
tems would be substituted for the single larger vessel.
Otherwise the equipment in the plant would be the
same. The advantage would be that the plant could con-
tinue to operate at part load while one or two modules
were down for maintenance. We were sufficiently im-
pressed by this capability to make the modular concept
the basis for the: design studies described in later sec-
tions of this report. No analysis was made of the opti-
mum size for a module. We simply decided for the pur-
poses of this study to provide four modules in our
1000-Mw(e) plant.
~ All our designs for MSBR plants have fuel and blanket
circulation systems that are separated from the steam
system by an intermediate coolant system. If the steam
system were coupled directly to the fuel salt system by
means of a steam generator, any leaks in the tubes of
the steam generator would result in steam or water
leaking into the fuel salt. Reactions between water and
fuel salt would not be violent, but corrosive hydrogen
fluoride would be generated, and uranium oxide would
precipitate in the salt. Also, special provisions would
have to be included in the design to prevent the fuel
circulation system from being raised to the high
pressure of the steam system, Molten sodium, helium,
and other coolants have been considered for use in the
coolant system, but we prefer a molten salt. Sodium
reacts with the fuel salt to generate considerable heat,
precipitate uranium, and raise the melting point of the
salt. Helium does not react with the salt but must be
used at high pressure in order to obtain a good heat
transfer coefficient in the primary heat exchanger. At
best the heat transfer coefficient with gas is con-
siderably less than can be obtained with sodium or salt
“and results in an undesirably high inventory of fuel salt
and fissionable uranium in the reactor system. The
TLiF-BeF, coolant salt used in the MSRE is a good
coolant, but it costs about $1400 per cubic foot, and its
melting point is about 840°F. We would prefer to have
a less exi)ensive cobli_ng’ sélt with a lower melting point.
The salt NaBF,-NaF (92-8 mole %) costs only about
~ $60 per cubic foot, melts at 725°F, and is a favored '