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ORNL-CF-53-9-84.txt
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ORNL
m FAES Wl
OAK RIDGE SCHOOL OF REACTOR TECHNOLOGY 5 g /
F. C, Vonderlage, Director
’ [_—’
"This document consists of &5 —_pages,
No..":..;."":i__ ofgfi._l_Zchcpies, Series,*fi.;..‘_"
Reactor Deasign and Feasibility Problem
¥ A REFLECTOR MODERATED, CIRCULATING FUEL, AIRCRAFT REACTOR"
Prepared by:
J. H. MacMillan, Group Chairman
C. B. Anthony
K. Guttmann
C. P, Martin
J. L. Munier
R. D. Worley
August 1k, 1953
# A REFIECTOR MDIERATE
Digtribution:
1. J. 3. MacMillian
2. B, Anthony
3. Futitmann
b, P, ¥artin
50 L. Munler
6o D. Worley
Mo Fox
8. Mills
9. Mann
10, . Welnberg
11. Zmola
12, ., Blizard
13. . Briggs
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19. . B. Larson
20. . N. Lyon
21. . C. Briant
22, . ¥, Frasas
23. . A, Swartoub
=
il OoHEER P E QR WO
W riters
Poppendisk
Cole
Livingston
Rickover
Bussard
Yonderlags
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Alexander
ey
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wh AR WARE abpiediad D
REACTOR"
hO-41 DLViSlO Raactor Development, AEC, Washingion
L2-45 Central Reseavch Idbravy
h6-51 CRSORT Files
52-132 Laroratory Racords
PREFACE
The program which has evolved at the Jak Ridge School of
Reactor Technoiogy consiste of two eemesteré of formal course instruc-
tion, followed by ten weeks given to reactor design studies. These
gtudies provide each student an opportunity of applying to a specific
but representative problem the principles and technfilogy which the
school attempts to impart. Individual student groups are chosen so as
to include men of the various engineering professions and scientific
fields in much the same pattern found in a typical reactor project.
This report is based on the study made by its authors while
they were studente in the 1952-53 session of QRSQRT@ It was made and
the report prepared in ten weeks. Obviocusly those weeks wvere diligently
spent. Even so 1t would be unreasonable to expect that the study
reported here is either definitive or free of defect in judgement. The
faculty and meny, perhaps all of the studente are convinced that the
project well served its pedagogical purpose. The report is published
for the value 1t has to those who are professionally engeged in the field,
Ag the authors have noted, several members of the Oak Ridge
National Laboratory gave generougly of their time and,knmwledgé” The
faculty Joins with the authors iu appreciation of that help. Most
particularly is acknowledged the adwvice and inspiration which the group
recelved from ite consultant, E. R. Mamn.
~ F. C, Vonderlage
e ‘
flgk‘for
-
ACKNOWLEDGEMENT S
This group wishes to express its appreciation to the members
of the CRSCRT faculty who presented the information which served as
the technical background for this study. Thanks are also extended to
all members of the Oak Ridge ANP group for their invaluable
assistance, patient consultation and cordial hospitality.
For his guidance and assistance. this group expresses its
appreciation to the group advisor, E. R, Mann, Particular thanks
are also extended to H. F. Poppendiek who made the flow experiment
possible and to A. H. Fox for his guidance on the nuclear aspecte
of the reactor,
;nf!ca
Acknowledgements
Tible AT Contents
List of Figures
Section 1
Section 11
hol
b3
A
L
section V
5.1
o R
W
5.3
Introduction
Summary
General Plent Design
Greneral Descriplion
t‘:j
esilgn Philosophy
T
Materis
€3
-
Yot
ffuel
Reflector
Moderator
Intermediate Heat Transfer Mediumr
Fabrication
Reactor Physics
Cross Sections
Sell-snielding
One Group, Two Regilon, Critiecslity Calculation
Two Group, Three flegion Calculation
Temperature Ceefficilent of Heactivity
Fission Product Handling
Excess Pael Reguirements
Einetics
4
o
N0 s 3
12
5
9
- Controls
5,10 ~ Btart Up
5.11 « Shut Down
Section VI - Reactor Englnesring
6.1
60
6.
Section VII
2
3
- Optimization
- Heat Transfer
6.2.1 = Germa Heating
6.2.2 - Internal Heat Transfer
6,2.3 - Reflector Cooling
6.2.4 - Primary Heat Exchanger
6.2.5 - NaOD Heat Exchanger
-~ Fuel Flow Experiment
- Shielding
Section VIII ~ Conclusions end Recommendations
Sectlion I -
Section X -
om0 W
10
References
Appendices
- Design Data
-
One Group, Two Reglion Data
Two Group Cross Section Weighting
Two Group, Three Region Data
Optimization
(ramma Heating
Core Heal Transfer
Primary Hesat Exchanger
NaCD Heat Exchangsr
Nomenciature
38
39
39
40
Lo
40
40
Ly
k9
53
5k
25
o7
29
61
63
63
67
10
n
73
76
71
78
Figure Number
1
2
O
10
11
12
13
14
LI15T OF FIGURES
Title
General Plant Layout
Schematic Drawing of the Fuel Tubes
Typical kgpe vs. Uranium Mass Curve
Characteristic Self-shielding Factors
Thermal Utilization Curves for Cylindrical
Fuel Tubes
Nuclear Approximation of the Screwball
Gamma Heating Distrifiution
Over-all Heat Transfer Coeffiecient vs,
NeOD Velocity
N20D lieat Transfer Coefficient vs, NaQD
Velocity
Temperature Variations Through the Core
Reflector Power Absorption Curve
Photograph of the Flow Experiment Apparatus
Shield Weight Curve
Ciyitical Determinant
oo
25
45
L7
48
50
52
56
58
30
I INTRODUGTION
The objective of this project was to apply the theoretical
information presented at ORSORT to the design of a reflector-
moderated, circulating fuel, aircraft reactor.
The scope of the investigation was limited primarily to
an analytical evaluation, although a minor flow experimeni was
performed .
This design study has been limited to the reactor; the
propulsion system has not been considered.
IT SUMMARY
A preliminary feasibility study of a 200 MW reflector moderated,
circulating fuel, aircraft reactor is presented. The Screwballm core
configuration as presently conceived consists of:
1) A spherical shell beryllium reflector
2) ARE tybe fluoride fuel in helical tubes arranged in
annular form
3) NaOD moderator and reflector coolant
In an attempt to justify the use of fuel tubes, an experimental
investigation of the flow in a model helical tube was conducted.
The reactor analysis was conducted on a two group, three region
basis. The nuclear cross sections were appropriaztely weighted and
judiciously applied so that the results compared favorably with the
multi-group machine calculations.
The reactor presented is believed to be conservative and appears
to be feasible, The fundamental limitation is the 1250°F maximum wall
temperature tor prevent excessive NaOD corrosion. Large NaOD flow rates
and ample flow guidance are required to minimize corrosion. If the
corrosion limit can be raised, the use of NaQOD as moderator and
coolant has greater potential.
Helical fuel tubes ares recommended to reduce the uncertainties
of unstable flow in high power-=density reactors. The engilneering
complexities introduced by their use are justified for controlled flow.
* The resctor described in this report will be called the "Screwball®
(the Fireball with = new twist). .
ITIT GENEBAL PLANT DESIGN
3.1 General Description
The Screwball is a spherical, reflector moderated, eirculating
fuel reactor. The fuel enters the gore at the north pole and flows
downward through six 3.5 inch I.D. inconel tubes. Five of these tubes
are wrapped in a variable pitch helix to form a spherical annulus of
fuel and the sixth tube passes through the center of the sphere forming
a helix of smaller diameter, See Figures 1 and 2. In returning the
fuel flows over NsK cooled tubes in the primary heat exchanger which is
wrapped in a spherical annulus surrounding the beryllium reflector.
The beryliium reflector has the form of a spherical shell with holes at
the north and south poles for entry of the fuel tubes. Sodium deuteroxide
flows downward through the spherical cavity in the beryllium and surrounds
the fuel tubes, hence functioning as a moderator "island". The NaQOD
returns to the top through 0.23 inch diemeter holes drilled in the
reflector and through a spherical cavity outside the reflector thereby
removing the heat preduced in the reflector., The NaOD then passes through
& heat exchanger and is pumped back through the core,
The intermediate heat transfer medium, NaK, returning from the
propulsion system passes through the sodium deuteroxide heat exchanger
and then through the primary heat exchanger. This system uses only one
intermediate heat transfer medium and eliminates the necessity of
additional radiators for subcooling a portion of the NaK as proposed for
the Fireball. However, a control system is required which will keep the
return NaK temperature constant., If the temperature rises, the NaOD will
be insufficlently cooled and excessive corrcsion may result. At return
FUEL TUBES
- GUIDE YANES
| = ==
GAS CPESSURE
?
I{g
DEUTERIUM L_jl_— ;.\i\
MAK INLET O :
i
1
’L
EXCHANGER
FIGURE |
SCREWBALL
GENERAL LAYOUT
APBPROKIMATE SCALE ~ 4 SIRE
30~
/o
NaQD HEAT __/
- AA
L~ BB
BORON LAYERS
~_ 7
’_KPRESSUEE SHELL
( =—FUEL DRAIN
- NaOD DENN
Dwm'n, Hamre
- 0
UNCLASSIEIED
DW7.#2—3M"7
FUEL IN
FUEL OQUT
OWG, BY C.PM.
SCHEMATIC DRAWING
OF FUEL TUBES
-11-
temperatures below 200°F,, the fuel will freeze in the primary heat
exchanger, With its inherent simplicity, the use of a single transfer
medium warrants further investigation. Figure 1 is & drawing of the
Screwball system, and a tabulation of design dasta is contained in the
Appendix 1.,
3.2 Desipn FPhilosophy
A brief survey of NEPA, ANP, H, K. Ferguson, and Technical Advisory
Board reports indicated that homogeneous reactors held the greatest
potential for efficient nuclear propelled flight. Since little information
is available on a combined hydroxide of lithium and sodium (the most obvious
candidate for a high temperature homogeneous reactor fuel)} the circulating
fuel type reactor was chosen as an intermediate step between fixed fuel
elements and the homogeneous type fuel. The large heal tranzfer surface
required in fixed fuel reactors is removed from the core in circulating
fuel reactors and the potential simplicity of homogeneous reactors is
retained., The moderating propertlies of the uranium bearing, fused salts
are generally poor, but employing thick, . efficient reflectors enables the
construction of a small high power reactor.
Having chosen a reflector moderated, circulating fuel type reactor,
a nore detailed investigation was initiated on the Fireball as described in
Referenca 2, Investigation of the Fireball design parameters yielded the
following five problems which appeared to warrant basic design changes or
modifications:
1. Eigh power density
2. Questionable fuel flow patterns
3. VPossibility of pressure surges
12
L. Cooling the Be "igland"
5. Self-shielding in the fuel
The Screwball eliminates or reduces the magnitude of each of
these problems except pressure surges. To achieve these ends compromises
in simplicity and resctor size have been medes however, the increase in
shield weight over the 22.5 inch core is less tham 10%. It is believed
that this reactor has a real potential for alreraft application, and as
such warrants further investigation.
The controllability of a high power density reactor has been neither
proven nor disproven. E. R, Mann states that controlling a reactor in which
the fuel temperature rise in the core exceeds 2000°F. per second will be
difficult and somewhat doubiful. To be more conservative, a power density
of 2.5 K¥/cc (1070°F. per second) has been chosen for this reactor.
With such rapid increases in fuel temperature only short lived flow
instabilities or eddies can be tolerated in the fuel., The use of fuel
tubes in the Screwball has greatly reduceé the uncertainty of sustained
instabilities in the fuel region. Aabrief gqualitive experiment varifying
stable flow through helical pipes is described in Section 6.3.
Pressure surges result from rapid density changes due to temperature
variations which occur in eddies of lengthy duration, or from the
instentaneous introduction of a cold slug of fuel. A step decrease in
temperature is difficult to visualize in a cireculating fuel reactoer,
Pressure surge calculations have been made on the Fireball assuming stagnant
fuel in the core and a step increase in k of 1% throughout the core.
These assumptions are both conservative since neither condition is likely to
oceur in the reactor. Based on these assumptions the resulting pressure
-] 3w
surge is not expected to exceed 150 psi.. As a result of the more
tortuous expansion path out of the core, pressure surges in the
Screwball are expected to be larger. However, the fuel tubes in the
Serewball will withstand pressures of 200 psi and no difficulty from
this phenomenon is antieipated.,
The beryllium central "island" in the Fireball reactor requires
ccoling to remove the heat generated by neutron moderation and gamma ray
attenuation. The density of heat generation is 100 to 200 watts/cc, and
its removal will require a large number of coolant tubes. The beryllium
hes been replaced in the Screwball by a circulating "island® of NaOD,
However, the problem of NaOD corrosion has been introduced. As indicated
in Section 6.2.2, no stagnant or low velocity layers in NaOD can be
tolerated next to the hot fuel tubes or containing shell.
The self-shielding effect, as described in Section 5.2, for the
3.5 inch diameter tubes of the Screwball should be less severe than for
the spherical fuel annulus in the Fireball.
] Lo
IV MATERIALS
4.1 Fuel
The proposed fuel for the Screwball is a fused salt containing
50 mole percent NaF, A7 mole percent ZrFA, and 3 mole percent enriched
UF&. This fuel is similar to that prqposed for the ARE and was chosen
because considerable information is availsble on its
physical and chemical properties. To relax the limitation on the
temperature of the returning NaK (Section 3.1}, a fuel with a lower melting
point would be desirable. Inconel will be used as the fuel containing
material.
4.2 Reflector
The reflector has two functions; moderation and shielding., Be is
a good moderator. Its moderating ratio is 159 compared to 170 for carbon,
In addition, it serves as an excellent shield due to its high atomic
density and small age. The fast neutron leakage for a given reflector
thickness is much smaller for beryllium than for sybstances. such as NaOD,
BeC, graphite and BeO apgregate. (Reference 2, Figure 7). Hence,
beryllium has been chosen for the Screwball reflector.
4.3 Moderator
A fluid moderator with 2 low vapor pressure al elevated temperature
was desired., Their high wapor pressures eliminated the possibility of
using light or heavy water. Hydroxides were then considered,
The diffusion length of a hydroxide is very small relative to its
age. Hencé, a hydroxide in the core of the Screwball would serve &s a
sink for fast neutrons rather than as a moderator, Deuteroxides do not
have this undesirable nuclear property and should exhibit similar physical
-] 5
and corrosive properties. Therefore, 110D ; NaOD and combinations of
both were considered., The double isotopic separation eliminated LiOD
from serious considerationi NaOD was chosen for the core moderstor,
Na0D also serves as the coolant for the reflector., It is a better
moderator than sodium (the proposed Fireball reflector coolant) so that
the Screwball reflector should be a more effective shield. However, the
macroscopic cross section for thermal neutrons is larger for NaOD than for
godium, The slight difference in absorption does not warrant cohsidering
the additional complexity of a separate sodium system for the Serewball,
BMI has made a survey of containing materials for NaOH at
elevated temperatures (Reference 23). Graphite, silver and nickel were
the most salisfactory of the materials tested, Nickel was chosen for the
Screwball on the basis of ease of cladding and electroplating and tolerable
neutron cross section. The corrosion mechanism of NeOH on nickel is
reported in Reference 4.
2 NaOH + Ni = NephiOp H,
N&2O @Ni()
The reaction equilibrium is temperature sensitive resulting in
mass transfer of nickel from hot regions to adjacent colder surfaces,
The corrosion can be suppressed by hydrogen pressure over the NaOH,
The corrosion mechanism for NaOD is expected to be gimilar to
that for NaOH, but the degree and temperature dependance of the corrosion
are unknown, For this study, the temperature Ilimitation for NaOb
corrosion of nickel is assumed the same as for NaOH,
According to Reference 3, corrosion of nickel by stagnant NaCH is,
~16~
1) not néticable at 1000°F
2) small at 1250°F and would be tolerable for
alireraft applications
3) excessive at 1500°F
A 1imiting wall temperature of 1250°F and a deuterium gas
pressure in the NaOD expansion tank of two to three atmospheres are
proposed for this reactor.
4oL Intermediate Heat Transfer Medium
A near eutectic alloy of sodium and potassium, 56 weight percent
Na and 44 weight percent K, has been chosen as the intermediate heat
transfer medium. As is typical of liquid metals, this alloy has excellent
heat transfer properties and also has a low melting point (66°F), The
main disadvantage of NaK is the induced radiation resulting from neutron
bombardment in the primary heat exchanger.
4.5 Fabrication
The proposed methods for fabricating the primary heat exchanger,
punps and beryllium reflector are the same as those described in
Reference 2, Ni will be substituted for chromium in the reflector.
Bending the fuel tubes is possible (Reference 5), with the use
of a cermet internal mandrel.
The NaOD heat exchanger is standard, welded shell and tube
construction.
The entire system will be welded, Reference 6 states that welds
in nickel for 1000°F NaOH corrosion tests were made with no unusual
difficulty. Inconel welding presents no major e¢omplications.
The fabrication sequence has not been fully considered in the layout
of Pigure 1. Modifications may be required to facilitate assembly of parts.
=17
V REACIOR PHYSICS
5.1 Cross Sections
The cross sections used for nuclear calculations in this report
are based on current ANP data.
5.2 3elf-shielding
The application of diffusion theory in Reactor design, yields at
best only a reasonable gpproximetion of the nuclear characteristics of
homogeneous systems. The Screwball is a heterogeneous rezctor which has
been homogenized for the purpose of expediting the nuclear calculations.
This fact makes it necessary to correct the diffusion eguations by lntroducing
a parameter commonly referred tc as the self-shielding factor, F. This
factor accounts for the local depression of the neutron flux within the fuel
region, which in turn results in decreased thermal utilization of the fuel
Two major disadvanbtages result from self-shielding. First, more fuel is
required than for a homogeneous reactor of the same proportions: and
second, the negative temperature coefficient is not as large. As seen in
Filgure 3, a smaller change in k pe results from the removal of an equal
mass of uranium for a reactor with a greater uranium investment.
Figure /4 depicts estimated values of F vs. fuel tube diameter at
various reactor operating temperatures., The calculations were based on
the method set forth in Reference 7. To apply the method one must know
2 and % of each constituent, the atomic densities in the fuel tube and
its diameter, and the variation of f with 2By as shown in Figure5~
From these data calculate,
18-